- Colin Farrell Character (Jesse James)
- Scott Caan Character (Cole Younger)
- Ali Larter Character (Zerelda 'Zee' Mimms)
- Gabriel Macht Character (Frank James)
- Gregory Smith Character (Jim Younger)
- Kathy Bates Character (Ma James)
- Timothy Dalton Character (Allan Pinkerton)
- Harris Yulin Character (Thaddeus Rains, President Rock Northern Rail Road)
- Will McCormack Character (Bob Younger)
- Ronny Cox Character (Doc Mimms, Zee's Dad)
- Terry O'Quinn Character (Rollin H. Parker - Rains' Gopher)
- Nathaniel Arcand Character (Comanche Tom)
- Ty O'Neal Character (Clell Miller)
- Joe Stevens Character (Loni Packwood)
- Barry Tubb Character (Captain Malcolm)
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